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adf:tpatheory

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Assuming two degenerate photons that are linearly polarized, the TPA cross section (σ$_{TPA}$) can be calculated using the imaginary part of the third-order response property as

where α$_f$ is the fine structure constant, and the σ$_{TPA}$ unit is given as Göppert-Mayer (1 GM = 10$^{−50}$ cm$^4$ s photon$^{−1}$). The integer value N is related to the experimental setup, and in this work, N = 4 is used for all simulated TPA spectra.

参考文献

  • Silverstein, D. W.; Jensen, L. J. Chem. Phys. 2012, 136, 064111.
  • Beerepoot, M. T. P.; Friese, D. H.; List, N. H.; Kongsted, J.; Ruud, K. Phys. Chem. Chem. Phys. 2015, 17, 19306−19314
adf/tpatheory.1582010841.txt.gz · 最后更改: 2020/02/18 15:27 由 liu.jun

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